TY - JOUR
T1 - Two-Dimensional Carbon Graphdiyne
T2 - Advances in Fundamental and Application Research
AU - Zheng, Xuchen
AU - Chen, Siao
AU - Li, Jinze
AU - Wu, Han
AU - Zhang, Chao
AU - Zhang, Danyan
AU - Chen, Xi
AU - Gao, Yang
AU - He, Feng
AU - Hui, Lan
AU - Liu, Huibiao
AU - Jiu, Tonggang
AU - Wang, Ning
AU - Li, Guoxing
AU - Xu, Jialiang
AU - Xue, Yurui
AU - Huang, Changshui
AU - Chen, Chunying
AU - Guo, Yanbing
AU - Lu, Tong Bu
AU - Wang, Dan
AU - Mao, Lanqun
AU - Zhang, Jin
AU - Zhang, Yue
AU - Chi, Lifeng
AU - Guo, Wanlin
AU - Bu, Xian He
AU - Zhang, Hongjie
AU - Dai, Liming
AU - Zhao, Yuliang
AU - Li, Yuliang
N1 - Publisher Copyright:
© 2023 American Chemical Society
PY - 2023/8/8
Y1 - 2023/8/8
N2 - Graphdiyne (GDY), a rising star of carbon allotropes, features a two-dimensional all-carbon network with the cohybridization of sp and sp2 carbon atoms and represents a trend and research direction in the development of carbon materials. The sp/sp2-hybridized structure of GDY endows it with numerous advantages and advancements in controlled growth, assembly, and performance tuning, and many studies have shown that GDY has been a key material for innovation and development in the fields of catalysis, energy, photoelectric conversion, mode conversion and transformation of electronic devices, detectors, life sciences, etc. In the past ten years, the fundamental scientific issues related to GDY have been understood, showing differences from traditional carbon materials in controlled growth, chemical and physical properties and mechanisms, and attracting extensive attention from many scientists. GDY has gradually developed into one of the frontiers of chemistry and materials science, and has entered the rapid development period, producing large numbers of fundamental and applied research achievements in the fundamental and applied research of carbon materials. For the exploration of frontier scientific concepts and phenomena in carbon science research, there is great potential to promote progress in the fields of energy, catalysis, intelligent information, optoelectronics, and life sciences. In this review, the growth, self-assembly method, aggregation structure, chemical modification, and doping of GDY are shown, and the theoretical calculation and simulation and fundamental properties of GDY are also fully introduced. In particular, the applications of GDY and its formed aggregates in catalysis, energy storage, photoelectronic, biomedicine, environmental science, life science, detectors, and material separation are introduced.
AB - Graphdiyne (GDY), a rising star of carbon allotropes, features a two-dimensional all-carbon network with the cohybridization of sp and sp2 carbon atoms and represents a trend and research direction in the development of carbon materials. The sp/sp2-hybridized structure of GDY endows it with numerous advantages and advancements in controlled growth, assembly, and performance tuning, and many studies have shown that GDY has been a key material for innovation and development in the fields of catalysis, energy, photoelectric conversion, mode conversion and transformation of electronic devices, detectors, life sciences, etc. In the past ten years, the fundamental scientific issues related to GDY have been understood, showing differences from traditional carbon materials in controlled growth, chemical and physical properties and mechanisms, and attracting extensive attention from many scientists. GDY has gradually developed into one of the frontiers of chemistry and materials science, and has entered the rapid development period, producing large numbers of fundamental and applied research achievements in the fundamental and applied research of carbon materials. For the exploration of frontier scientific concepts and phenomena in carbon science research, there is great potential to promote progress in the fields of energy, catalysis, intelligent information, optoelectronics, and life sciences. In this review, the growth, self-assembly method, aggregation structure, chemical modification, and doping of GDY are shown, and the theoretical calculation and simulation and fundamental properties of GDY are also fully introduced. In particular, the applications of GDY and its formed aggregates in catalysis, energy storage, photoelectronic, biomedicine, environmental science, life science, detectors, and material separation are introduced.
KW - atomic catalysis
KW - controlled growth
KW - energy conversion
KW - graphdiyne
KW - intelligent device
KW - life science
KW - material separation
KW - two-dimensional carbon materials
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U2 - 10.1021/acsnano.3c03849
DO - 10.1021/acsnano.3c03849
M3 - Review article
C2 - 37471703
AN - SCOPUS:85166744975
SN - 1936-0851
VL - 17
SP - 14309
EP - 14346
JO - ACS Nano
JF - ACS Nano
IS - 15
ER -